3. The Silence of the Lambs
Clarice Starling, a young intelligent FBI trainee, has been sent to the Baltimore state hospital for the criminally insane to interview an inmate Dr. Hannibal-the cannibal- Lecter. A brilliant renowned psychiatrist turned infamous psychopathic serial killer. She must match wits with Lecterm, who has the darkest of all minds, and trust him to give her clues in the search for "Buffalo Bill". A nick name for a loose, unknown, unstoppable psychopathic serial killer.
4. Shutter Island
This Thriller is found in the psychological Thriller category, is made in 2010 and is based on Dennis Lehane's 2003 novel. Leonardo DiCaprio plays the main role, who is investigating a psychiatric facility on the titular island.
It's 1954, and up-and-coming U.S. marshal Teddy Daniels is assigned to investigate the disappearance of a patient from Boston's Shutter Island Ashecliffe Hospital. He's been pushing for an assignment on the island for personal reasons, but before long he wonders whether he hasn't been brought there as part of a twisted plot by hospital doctors whose radical treatments range from unethical to illegal to downright sinister. Teddy's shrewd investigating skills soon provide a promising lead, but the hospital refuses him access to records he suspects would break the case wide open. As a hurricane cuts off communication with the mainland, more dangerous criminals "escape" in the confusion, and the puzzling, improbable clues multiply, Teddy begins to doubt everything - his memory, his partner, even his own sanity.
Here are two websites, which shows a list of the best thrillers of all time, but they differ from each other, due to the different assessments they used.
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